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Abstract We report the nature of magnetic structure, and microscopic spin-spin correlations and their dependence on the underlying crystal structure of the geometrically frustrated layered spin-32 maple leaf lattice (MLL) antiferromagnet Na2Mn3O7 by a comprehensive neutron diffraction study. Crystal structural studies by x-ray and neutron diffraction reveal that the MLL layers (constituted by Mn3O72− units) are well separated by nonmagnetic Na layers.
a Department of Chemistry, Biological and Chemical Research Centre, University of Warsaw, ?wirki i Wigury 101, Warsaw, Poland b Department of Chemistry, University of Copenhagen, Universitetsparken 5, DK-2100 Copenhagen, Denmark E-mail: madsen@chem.ku.dk c Department of Chemistry and Biochemistry, University of Bern, Bern, Switzerland
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