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1. Introduction The feverish search for advanced materials acting as solid, temperature stable electrolytes in sustainable, electrochemical energy storage systems has reached an unprecedented level. (1,2) To date, we are still in the initial phase to understand and to identify the most important design strategies that lead to ultrafast ion dynamics in solids.
The bidentate N,O-ligands phenol-pyrazole (HL1), naphthol-pyrazole (HL2) and the commercially available ligand 5-methylphenol-benzotriazole (HL3) were used for the synthesis of novel iron(III) complexes. The mononuclear iron complexes [FeCl(L1)2] (1), [FeCl(L2)2] (2) and [FeCl(L3)2] (3) are stable to air and moisture, both in the solid state as well as in solution, while the dinuclear, µ-oxido bridged complex [{Fe(L1)2}2(-O)] (1a) is air sensitive.
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