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In this study, we present a new aprotic solvent, 2,4-dimethoxy-2,4-dimethylpentan-3-one (DMDMP), which is designed to resist nucleophilic attack and hydrogen abstraction by reduced oxygen species. Li–O cells using DMDMP solutions were successfully cycled. By various analytical measurements, we showed that even after prolonged cycling only a negligible amount of DMDMP was degraded.
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After many years of successful and disappointing results, the field of Li-O research seems to have reached an equilibrium state. The extensive knowledge that has accrued through advanced analytical studies enables us to delineate the weaknesses of the Li-O battery. It is now clear that the instability of the cell components toward the extreme conditions existing during cell operation, leads to early cell failure as well.
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