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Synopsis The assembly potential of sulfonato-thiacalix[4]arene was investigated in combination with Zn2+ and two proteins with distinct structural/chemical properties. Thiacalixarene-supported di- or penta-nuclear Zn species were obtained. These thiacalixarene/zinc complexes enabled protein assembly and crystallization via protein-calixarene complexation as well as metal-mediated interfaces.
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