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1 Introduction The family of layered thio- phosphates, such as CuInP2S6, CuCrP2S6, CuVP2S6, has garnered significant attention due to their unique polar properties as 2D van der Waals materials [1-4]. These compounds host a rich spectrum of ferroic orders, including ferro- and antiferroelectric [5], ferro- and antiferromagnetism [6], and extending to more exotic states such as polar bubbles [7] and altermagnetism [8].
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