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1 Introduction Flavin-dependent halogenases (FDHs) use FADH2, O2, and Cl− to generate HOCl, which travels down a 10 Å tunnel to halogenate aromatic substrates via electrophilic aromatic substitution [1-4] (Figure ). These bacterial and fungal biosynthetic enzymes are attractive for green chemistry applications because they regioselectively synthesize aryl halides under mild reaction conditions.
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