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Articles by Hatice Kasap
Solar Reforming of Biomass with Homogeneous Carbon Dots
Cover Picture Dr. Demetra S. Achilleos http://orcid.org/0000-0002-1146-7138 Christian Doppler Laboratory for Sustainable SynGas Chemistry, Department of Chemistry, University of Cambridge, Lensfield Road, Cambridge, CB2 1EW UK Present address: School of Chemistry, University College Dublin, Science Centre South, Belfield, Dublin, Ireland Search for more papers by this author Prof. James R.
Solar Reforming of Biomass with Homogeneous Carbon Dots
Abstract A sunlight‐powered process is reported that employs carbon dots (CDs) as light absorbers for the conversion of lignocellulose into sustainable H2 fuel and organics. This photocatalytic system operates in pure and untreated sea water at benign pH (2–8) and ambient temperature and pressure. The CDs can be produced in a scalable synthesis directly from biomass itself and their solubility allows for good interactions with the insoluble biomass substrates.
Photocatalytic Hydrogen Generation Coupled to Pollutant Utilization Using Carbon Dots Produced from Biomass
Photocatalytic Hydrogen Generation Coupled to Pollutant Utilization Using Carbon Dots Produced from Biomass Photocatalysis is deemed as an appealing strategy to exploit solar energy for simultaneous fuel production and pollutant utilization. However, current photocatalytic systems rarely couple both processes and suffer from restricted scalability and sustainability as they use toxic and/or ultraviolet light harvesters, combined with noble-metal co-catalysts under corrosive conditions.
Photoreforming of Non-Recyclable Plastic Waste over a Carbon Nitride/Nickel Phosphide Catalyst
RETURN TO JUST ACCEPTED MANUSCRIPTSPREVArticleNEXT Taylor Uekert Hatice Kasap Erwin Reisner LEARN ABOUT THESE METRICS Article Views are the COUNTER-compliant sum of full text article downloads since November 2008 (both PDF and HTML) across all institutions and individuals. These metrics are regularly updated to reflect usage leading up to the last few days. Citations are the number of other articles citing this article, calculated by Crossref and updated daily.
Electron Accumulation Induces Efficiency Bottleneck for Hydrogen Production in Carbon Nitride Photocatalysts
This study addresses the light intensity dependence of charge accumulation in a photocatalyst suspension, and its impact on both charge recombination kinetics and steady-state H2 evolution efficiency. Cyanamide surface functionalized melon-type carbon nitride (NCNCNx) has been selected as an example of emerging carbon nitrides photocatalysts because of its excellent charge storage ability.
Photoreforming of Lignocellulose into H2 Using Nanoengineered Carbon Nitride under Benign Conditions
Photoreforming of lignocellulose is a promising approach toward sustainable H generation, but this kinetically challenging reaction currently requires UV-absorbing or toxic light absorbers under harsh conditions. Here, we report a cyanamide-functionalized carbon nitride, NCNCN , which shows enhanced performance upon ultrasonication.
Solar-Driven Reduction of Aqueous Protons Coupled to Selective Alcohol Oxidation with a Carbon Nitride-Molecular Ni Catalyst System
Solar water-splitting represents an important strategy toward production of the storable and renewable fuel hydrogen. The water oxidation half-reaction typically proceeds with poor efficiency and produces the unprofitable and often damaging product, O . Herein, we demonstrate an alternative approach and couple solar H generation with value-added organic substrate oxidation.
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