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Articles by Ivana Borilovic
Three individually addressable spin qubits in a single molecule
Three individually addressable spin qubits in a single molecule† Ivana Borilovic, a Olivier Roubeau, b Boris Le Guennic, c Joris van Slageren, d Samuel Lenz,d Simon J. Teat e and Guillem Aromí *a Abstract An asymmetric bis-phenol-β-diketone (H4L) has been designed as a ligand programmed to promote the assembly of a molecular arrangement composed of three magnetically exchanged [NiCu] pairs, each exhibiting an S = 1/2 spin.
Self-assembly of a trigonal bipyramidal architecture with stabilisation of iron in three spin states
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Tandem Mn-I Exchange and Homocoupling Processes Mediated by a Synergistically Operative Lithium Manganate
Research Article In memory of Gérard Cahiez PDF ShareShare Abstract Pairing lithium and manganese(II) to form lithium manganate [Li2Mn(CH2SiMe3)4] enables the efficient direct Mn–I exchange of aryliodides, affording transient (aryl)lithium manganate intermediates which in turn undergo spontaneous C−C homocoupling at room temperature to furnish symmetrical (bis)aryls in good yields under mild reaction conditions.
Heterometallic 3d-4f Complexes as Air-Stable Molecular Precursors in Low Temperature Syntheses of Stoichiometric Rare-Earth Orthoferrite Powders
Four 3d–4f hetero-polymetallic complexes [Fe2Ln2((OCH2)3CR)2(O2CtBu)6(H2O)4] (where Ln = La (1 and 2) and Gd (3 and 4); and R = Me (1 and 3) and Et (2 and 4)) are synthesized and analyzed using elemental analysis, Fourier transform infrared spectroscopy, thermogravimetric analysis, and SQUID magnetometry. Crystal structures are obtained for both methyl derivatives and show that the complexes are isostructural and adopt a defective dicubane topology.
A bis-vanadyl coordination complex as a 2-qubit quantum gate
A bis-vanadyl coordination complex as a 2-qubit quantum gate† A new bis-hydroxyphenylpyrazolyl ligand, H4L, allows isolating and structurally characterizing vanadyl and titanyl dinuclear complexes (Bu4N)2[(MO)2(HL)2] (M = V, Ti). The weak dipolar coupling and relatively short quantum coherence of the divanadyl anions are optimal for a 2-qubit molecular architecture proposed to implement electron-mediated nuclear quantum simulations.
Synthetic, Structural and Magnetic Implications of Introducing 2,2'-Dipyridylamide to Sodium Ferrate Complexes
Using a transamination approach to access novel Fe(II) complexes, this study presents the synthesis, single crystal X-ray diffraction and magnetic characterisation of a series of new iron complexes containing the multifunctional 2,2-dipyridylamide (DPA) ligand using iron bis(amide) [{Fe(HMDS)2}2] and sodium ferrate [{NaFe(HMDS)3}?] (1) as precursors, (HMDS = 1,1,1,3,3,3-hexamethyldisilazide).
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