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Complex coacervates formed between oppositely charged polyelectrolytes play important roles in encapsulation, micelles, adhesives and coatings. By contrast, coacervates between a polyelectrolyte and small molecules are hard-to-form, and the underlying mechanism remains elusive. Here, a cationic polyelectrolyte polyamidoamine epichlorohydrin (PAE) was explored to form a coacervate with a small molecule (i.e., sodium 4-hydroxybenzene sulfonate, 4-HBSNa).
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