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Cellulose nanocrystals (CNC) were converted into a CO2-responsive composite nanomaterial by grafting poly(dimethylaminoethy methacrylate) (PDMAEMA) and poly(diethylaminoethyl methacrylate) (PDEAEMA) on its surface using a grafting-from approach via surface-initiated copper(0)-mediated polymerisation (SI-Cu(0)-ATRP). The Cu(0)-ATRP homopolymerisation kinetics of these monomers were first studied to determine suitable conditions to perform the grafting step.
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