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Note This paper was published ASAP on March 7, 2020, with errors in Eq 1 and the surrounding text, and in the Supporting Information description. These were corrected in the version published on March 11, 2020. In a recent set of articles,(1−6) we studied in detail the rotational and translational diffusion of solutes dissolved in different ILs as well as the mobility of constituent ions and their internal polar and apolar subcomponents.
When solutes are small compared to the size of the ions in an ionic liquid, energetic heterogeneities associated with charge enhanced (stiff) and charge depleted (soft) nanoenvironments are sampled. In a recent article [J. C. Araque et al., J. Phys. Chem. B 119(23), 7015-7029 (2015)], we explored large deviations from Stokes-Einstein translational diffusion caused by such a heterogeneity.
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