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Articles by Julia G. Knapp
Insights for controlling plutonium behavior in hydrochloric acid solutions
Insights for controlling plutonium behavior in hydrochloric acid solutions† Advancing understanding of aqueous chemistry for plutonium is important because it impacts energy production, environmental management, and national security. Unfortunately, plutonium's aqueous chemistry remains poorly characterized.
Uranyl Uptake into Metal-Organic Frameworks: A Detailed X-Ray Structural Analysis
Uranyl Uptake into Metal–Organic Frameworks: A Detailed X-Ray Structural Analysis Metal-organic frameworks (MOF) are a subclass of porous framework materials that have been used for a wide variety of applications in sensing, catalysis, and remediation. Among these myriad applications is their remarkable ability to capture substances in a variety of environments ranging from benign to extreme.
Evidence of a Uranium‐Paddlewheel Node in a Catecholate‐Based Metal-Organic Framework
Introduction Uranium is an element rich in oxidation states; reports exist of coordination complexes of uranium in every oxidation state between +1 and +6.1-8 Each oxidation state is of fundamental interest due to the associated unique behavior in several regimes.
Ethylene polymerization with a crystallographically well-defined metal-organic framework supported catalyst
Ethylene polymerization with a crystallographically well-defined metal–organic framework supported catalyst† Timothy A. Goetjen, ab Julia G. Knapp, a Zoha H. Syed, ab Ryan A. Hackler, b Xuan Zhang, a Massimiliano Delferro, b Joseph T. Hupp *a and Omar K.
MOF-enabled confinement and related effects for chemical catalyst presentation and utilization
MOF-enabled confinement and related effects for chemical catalyst presentation and utilization Jian Liu, a Timothy A. Goetjen, ab Qining Wang,a Julia G. Knapp, a Megan C. Wasson, a Ying Yang,a Zoha H. Syed, ab Massimiliano Delferro, b Justin M. Notestein, c Omar K. Farha ac and Joseph T.
Electron transitions in a Ce(III)-catecholate metal–organic framework
Electron transitions in a Ce(iii)-catecholate metal–organic framework† Julia G. Knapp, a Debmalya Ray,b Paul B. Calio,c Megan C. Wasson, a Thais R. Scott,c Laura Gagliardic and Omar K.
Stabilization of Photocatalytically Active Uranyl Species in a Uranyl-Organic Framework for Heterogeneous Alkane Fluorination Driven by Visible Light
When photoactivated, the uranyl ion is a powerful oxidant capable of abstracting hydrogen atoms from nonactivated C–H bonds. However, the highly reactive singly reduced [UVO2]+ intermediate is unstable with respect to disproportionation to the uranyl dication and insoluble tetravalent uranium phases, which limits the usage of uranyl ions as robust photocatalysts.
Single crystal structure and photocatalytic behavior of grafted uranyl on the Zr-node of a pyrene-based metal-organic framework
Single crystal structure and photocatalytic behavior of grafted uranyl on the Zr-node of a pyrene-based metal–organic framework† Julia G. Knapp, a Xuan Zhang, a Tatyana Elkin, b Laura E. Wolfsberg, c Sylvia L. Hanna, a Florencia A. Son, a Brian L. Scott *b and Omar K.
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