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Abstract Organosulfur compounds are important constituents of atmospheric aerosols and have been extensively investigated through field observations, laboratory experiments, and atmospheric modeling. However, the mechanisms underlying their formation and atmospheric abundance remain incompletely understood. Ubiquitous in the atmosphere, micrometer-sized droplets provide unique interfacial reaction environments that may facilitate organosulfur formation.
3.2 Variation in the Vertical Structure of SLB A 15-year simulation of SLB was conducted using the WRF model with BASE experiment settings described in Section 2.2 to investigate the long-term variability mechanism in SLB in Tianjin. The simulated variations in the number of SLBD were generally in agreement with observations with a correlation coefficient of 0.91. The least number of SLBD was observed in 2011 (Figure S2).
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