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1 Introduction The groundbreaking contributions to enantioselective Diels–Alder and aldol reactions have established asymmetric organocatalysis [1-4] conceptually and in its broad synthetic applications as a cornerstone of modern asymmetric catalysis. List's L-proline- and MacMillan's amino acid-derived imidazolidin-4-one organocatalysts, proved to be a universal platform for many different applications.
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