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Lucy Jenkins

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Articles by Lucy Jenkins

Catalytic Dinitrogen Reduction to Ammonia at a Triamidoamine-Titanium Complex

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By Laurence R. Doyle, Ashley J. Wooles, Lucy Jenkins, Floriana Tuna
| Arthritis & Rheumatology Verified
Catalytic reduction of N to NH by a Ti complex has been achieved, thus now adding an early d‐block metal to the small group of mid‐ and late‐d‐block metals (Mo, Fe, Ru, Os, Co) that catalytically produce NH by N reduction and protonolysis under homogeneous, abiological conditions. Reduction of [TiIV(TrenTMS)X] (X=Cl, 1A; I, 1B; TrenTMS=N(CH CH NSiMe ) ) with KC affords [TiIII(TrenTMS)] (2).
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Angewandte Chemie International Edition

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By Laurence R. Doyle, Ashley J. Wooles, Lucy Jenkins, Floriana Tuna
| pericles.pericles-prod.literatumonline.com
Catalytic reduction of N to NH by a Ti complex has been achieved, thus now adding an early d‐block metal to the small group of mid‐ and late‐d‐block metals (Mo, Fe, Ru, Os, Co) that catalytically produce NH by N reduction and protonolysis under homogeneous, abiological conditions. Reduction of [TiIV(TrenTMS)X] (X=Cl, 1A; I, 1B; TrenTMS=N(CH CH NSiMe ) ) with KC affords [TiIII(TrenTMS)] (2).
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Catalytic Dinitrogen Reduction to Ammonia at a Triamidoamine‐Titanium Complex

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By Stephen Liddle, Laurence R. Doyle, Ashley J. Wooles, Lucy Jenkins
| Arthritis & Rheumatology Verified
We report unprecedented catalytic reduction of N2 to NH3 by a molecular Ti complex, thus now adding an early d‐block metal to the small group of mid‐ and late‐d‐block metals (Mo, Fe, Ru, Os, Co) that are capable of executing catalytic production of NH3 by N2 reduction and protonolysis under homogeneous, abiological conditions. Under Ar, reduction of [TiIV(TrenTMS)X] (X = Cl, 1A; I, 1B; TrenTMS = N(CH2CH2NSiMe3)3) with 1 equivalent of KC8 affords [TiIII(TrenTMS)] (2).
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