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Abstract Solution processing remains the dominant route to high-performance perovskite/silicon tandems, but it remains challenging to simultaneously achieve industrial scalability and long-term reliability.1-3 Thermal evaporation is more industrially viable, yet it has not been successfully demonstrated for large-area perovskite/Si tandems, largely due to the thermal degradation of formamidinium iodide (FAI) during high-temperature evaporation.
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