A series of new homo- and heteroleptic gallium ketoiminate compounds, namely, tris[4-[2-(ethoxyethyl)imino]-2-pentanone] gallium(iii) [Ga(eeki)3] [1], tris[4-[3-(methoxypropyl)imino]-2-pentanone] gallium(iii), [Ga(mpki)3] [2], tris[4-[3-(methoxyethyl)imino]-2-pentanone] gallium(iii), [Ga(meki)3] [3], dichloro[4-[(isopropyl)imino]-2-pentanone] gallium(iii) [Ga(ipki)Cl2] [4], bisdimethylamido[4-[(isopropyl)imino]-2-pentanone] gallium(iii) [Ga(ipki)(NMe2)2] [5] and...