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Single-component organic conductors based on delocalized hydrocarbon π-radicals exhibit unique electrical, magnetic, and optical properties desirable for advanced organic electronics [1-5]. Odd alternant hydrocarbons (OAHs) are proposed to be excellent candidates for organic metal and superconductors [6], but they typically possess a narrow band width (W) and large on-site Coulomb repulsion energy (U), leading to a Mott insulating state [7-9].
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