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Articles by Mathieu Lizee
Disentanglement of interfacial electric fields and electrochemical potential gradients reveals a multidimensional kinetic landscape
Abstract Electrochemical reactions occur at solid–liquid interfaces, where the applied electrochemical potential gradient can act as thermodynamic driving force but can also induce interfacial polarization. A key question has long been how local changes in the chemical potentials of the electrons and the associated excess charge and electric fields impact catalyst kinetics.
Architecting mechanosensitive nanofluidic transport in graphite nanoslits
Abstract INTRODUCTION RESULTS DISCUSSION MATERIALS AND METHODS Acknowledgments Supplementary Materials REFERENCES Information & Authors Metrics & Citations View Options References Figures Tables Media Share Abstract Mechanosensitive ion transport plays a central role in enabling living systems to perceive and adapt to their environment through the deformation of soft, embedded ion channels.
Correlating Equilibrium Excess Charge with the Kinetics of the Multi-Step Hydrogen Evolution Reaction in Alkaline Media Click to copy article link Article link copied!
A century of double-layer theory (1−3) established how excess charge is stored and screened on ideally polarizable interfaces, but the understanding of the impact on the kinetics remains poor. Conway (4,5) and others (6,7) emphasized the importance of electric fields that could impact the solvation kinetics and other processes inside the double layer, but these effects were largely relegated to a narrow range of reactions.
Anderson transition symmetries at the band-edge of a correlated Sn/Si monolayer - Communications Physics
Abstract Anderson localization is predicted to enhance the critical temperature of disordered superconductors. Despite a huge body of theoretical work based on non-linear sigma models, experiments are lacking to understand correlated electrons in disordered potentials. In this study, we investigate a tin monolayer on silicon, a material known for its likely antiferromagnetic Mott-correlated ground state.
Anomalous friction of supercooled glycerol on mica - Nature Communications
Abstract Although friction of liquids on solid surfaces is traditionally linked to wettability, recent works have unveiled the role of the solid’s internal excitations on interfacial dissipation. In order to directly evidence such couplings, we take advantage of the considerable variation of the molecular timescales of supercooled glycerol under mild change of temperature to explore how friction depends on the liquid’s molecular dynamics.
Local density of states fluctuations in a two-dimensional superconductor as a probe of quantum diffusion
Abstract The interplay of superconductivity and disorder generates a wealth of complex phenomena. In particular, the peculiar structure of diffusive electronic wave functions is predicted to increase the superconducting critical temperature in some range of disorder. In this work, we use an epitaxial monolayer of lead showing a simple band structure and homogeneous structural disorder as a model system of a two-dimensional superconductor in the weak-antilocalization regime.
Strong Electronic Winds Blowing under Liquid Flows on Carbon Surfaces
Abstract Solid-liquid interfaces display a wealth of emerging phenomena at nanometer scales, which are at the root of their technological applications. While the interfacial structure and chemistry have been intensively explored, the potential coupling between liquid flows and the solid’s electronic degrees of freedom has been broadly overlooked up till now.
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