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Metal nanoparticles supported on a nonconductive oxide undergo pH-dependent spontaneous polarization Yogesh Surendranath, Thejas S. Wesley, Max Huelsey, Karl S. Westendorff, Noah B. Lewis, Ethan Crumlin and Yuriy Roman-Leshkov Abstract Electrochemical polarization, which often plays a critical role in driving chemical reactions at solid-liquid interfaces, can arise spontaneously through the exchange of ions and/or electrons across the interface.
Quantum Yield Enhancement in Photocatalytic HCOOH Decomposition to H2 under Periodic Illumination Sieshing Wong, Max Huelsey, Hua An and Ning Yan Abstract Despite numerous studies on controlled periodic illumination to improve the quantum yield of photocatalytic reactions, debates still exist on the nature of the enhancement effect. Here, we report the promotion of HCOOH dehydrogenation over TiO2-supported noble metal photocatalysts using periodic illumination.
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