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Abstract Silicon is widely regarded as one of the most promising anode materials for next-generation solid-state lithium-ion batteries because of its ultrahigh theoretical capacity and low lithiation potential. However, its practical application remains hindered by severe volume variation, unstable interphase evolution, and progressive loss of solid–solid contact during cycling.
Abstract Silicon is one of the most attractive anode materials for all-solid-state batteries (ASSBs) because of its high theoretical capacity, low lithiation potential, and abundance. Over the past 2 decades, silicon-anode research in ASSBs has evolved from thin-film model systems to nanostructured three-dimensional electrodes, powder-pressed composite architectures, integrated nanosheet-based cells, and, more recently, high-loading application-oriented designs.
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