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Abstract Hydration critically governs the physicochemical behavior of solutes in both the aqueous bulk and interfacial environments. As typical chaotropic Hofmeister ions, weakly hydrated anions (WHAs) can reshape hydration structures and accumulate at water–hydrophobe interfaces. Notably, WHAs paradoxically suppress the solubility of certain small-molecule monomers in water while enhancing that of chemically analogous polymers.
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