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Abstract Metal-halide perovskites offer high optoelectronic performance but translating laboratory efficiencies into controllable, reproducible processes remains challenging. Perovskite crystallization is tracked by in situ multiwavelength absorption to show that coherent, layer-by-layer conversion of low-n intermediates to three-dimensional perovskite, quantified by a transformation index (TI), correlates with device quality.
Conflict of Interest The authors declare no conflict of interest. Supporting Information Filename Description adma202410395-sup-0001-SuppMat.pdf2.7 MB Supporting Information adma202410395-sup-0002-VideoS1.mp49.3 MB Supplemental Video 1 adma202410395-sup-0003-VideoS2.mp46.1 MB Supplemental Video 2 adma202410395-sup-0004-VideoS3.mp411.5 MB Supplemental Video 3 References 1 N. R. E. L.
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