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Articles by Simone Gillbard
Nickel‐Catalyzed Arylative Cyclizations of Alkyne‐ and Allene‐Tethered Electrophiles using Arylboron Reagents
Abstract The use of arylboron reagents in metal-catalyzed domino addition-cyclization reactions is a well-established strategy for the preparation of diverse carbo- and heterocyclic products. Recent studies have demonstrated nickel catalysis is highly effective in these reactions, in many cases offering unique reactivity and access to products that might otherwise not be readily available using other metal catalysts.
Enantioselective nickel-catalyzed anti-arylmetallative cyclizations onto acyclic electron-deficient alkenes
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Synthesis of multisubstituted pyrroles by nickel-catalyzed arylative cyclizations of N-tosyl alkynamides
S. M. Gillbard, C. Chung, S. N. Karad, H. Panchal, W. Lewis and H. W. Lam, Chem. Commun., 2018, Accepted Manuscript , DOI: 10.1039/C8CC06649C If you are not the author of this article and you wish to reproduce material from it in a third party non-RSC publication you must formally request permission using Copyright Clearance Center. Go to our Instructions for using Copyright Clearance Center page for details.
Ligand and solvent control of selectivity in the C-H activation of a pyridylimine-substituted 1-naphthalene; a combined synthetic and computational study
The pyridylimine-substituted 1-naphthalenes, 2-(1-C10H7)-6-{CR=N(2,6-i-Pr2C6H3)}C5H3N (R = Me HLMe, H HLH), react with Na2[PdCl4] in acetic acid at elevated temperature to afford either ortho-C-Hnaphthyl activated (LMe)PdCl (2ortho) or the unactivated adduct (HLH)PdCl2 (1b). Alternatively, 1b and its ketimine analogue (HLMe)PdCl2 (1a), can be prepared by treating (MeCN)2PdCl2 with either HLMe or HLH in chloroform at room temperature.
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