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In this study, we introduce a novel setup for directly tracking the electrochemically active area during the stripping of a Li-metal electrode. Figure 1 depicts our method to leverage an optically transparent single-crystal LLZO electrolyte and directly observe Li stripping under reflected light. Using an LLZO Li-ion conductor ensures that no secondary interphase is present at the Li|SE interface, as pristine Li metal and LLZO do not react.
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