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Abstract The electrochemical reduction of CO2 offers a promising route to valuable fuels; however, stable performance is hindered by gas–liquid transport limitations in the cathode gas diffusion electrode (GDE), which are directly affected by GDE compression. Here, we showed that operating an alkaline zero-gap CO2 electrolyzer at a compression ratio (CR) of 10% achieved higher CO faradaic efficiency compared to CR = 20% and 30%.
Dehydrogenating methylcyclohexane (MCH) as a liquid organic hydrogen carrier offers a promising method for producing stored hydrogen. However, the transport properties of the gas diffusion layers (GDLs) in dehydrogenation cells (D-cells) have not yet been optimized for high reactant saturation at the GDL-catalyst layer (CL) interface, which is crucial for increasing hydrogen production.
1 Introduction Polymer electrolyte membrane water electrolyzers (PEMWEs) are a promising technology for green hydrogen generation. In an operating PEMWE, electricity (which can be obtained from renewable sources) is used to electrochemically convert water into hydrogen and oxygen gases.[1-4] A key component of the PEMWE stack that facilitates these electrochemical reactions is the porous transport layer (PTL).
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