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Interatomic Coulombic decay (ICD) is an efficient electronic decay mechanism of electronically excited atoms and molecules embedded in an environment. For the series of isoelectronic Na +, Mg 2+, and Al3+ ions in aqueous solution, ultrashort ICD lifetimes of 3.1 fs, 1.5 fs, and 0.9 fs, respectively, were observed experimentally.
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