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Xianglong Du

As seen in: Nature, Royal Society of Chemistry
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Articles by Xianglong Du

Ion-disrupted hydrogen-bond networks enable fast water transport under two-dimensional confinement

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By Mingyang Xia, Xianglong Du, Canbin Wang, Jinguo Liu, Zhihua Zhou, Yao-Hui Wang, Fujie Tang, Sheng Hu, Ying-Ru Qiu
| Nature Verified
Abstract Water transport under nanoscale confinement often exhibits anomalously high flow rates that defy classical hydrodynamic descriptions. While such behavior is commonly analyzed assuming pure water, confined water under realistic conditions inevitably contains dissolved ions. How ion-water interactions reshape hydrogen-bond networks and regulate nanoscale water transport therefore remains poorly understood.
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Water at electrode-electrolyte interfaces: combining HOD vibrational spectra with ab initio-molecular dynamics simulations

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By Jiabo Le, Pavithra Gunasekaran, Xianglong Du, Andrew Burley
| Royal Society of Chemistry Verified
Water at electrode-electrolyte interfaces: combining HOD vibrational spectra with ab initio-molecular dynamics simulations We have undertaken a vibrational study of the structure of interfacial water and its potential dependence using H2O:D2O mixtures to explore the O-H and O-D stretching modes of HOD as well as the bending modes of HOD and H2O. Due to the symmetry reduction, some of the complexity characteristic of the vibrational spectrum of water is removed in HOD.
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