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Abstract Thermal evaporation of perovskite films holds considerable promise for the scalable manufacturing and pixel patterning of perovskite light-emitting diodes (PeLEDs). However, the performance of evaporated PeLEDs remains inferior to their solution-processed counterparts due to the lack of effective strategies to regulate perovskite crystallization during vacuum deposition. Here we address this challenge and achieve precise control over crystallization pathways.
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