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Graphical Abstract Carbothermal shock (CTS) method with high heating and cooling rates, high temperatures (up to ≈2200 °C), and ultrafast reaction times of ≈20 s is utilized for recycling spent cathode materials. Li can be selectively leached through water leaching with an efficiency of >90 %. Ni, Co, and Mn are recovered by dilute acid leaching with efficiencies >98 %.
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