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The electrostatic field of dielectric cavity is powerful to modulate the confined metal clusters in many aspects. Here we report the catalytic properties of Ptn clusters confined in X-zeolite cages are strongly tuned by altering the zeolitic field, which is achieved by using different cations (Na+, Cs+, Ca2+ or La3+) to balance the negative framework of the zeolite.
The hydrogenation of phenol to cyclohexanone is an important industrial reaction and supported palladium catalysts are the most popular catalysts applied nowadays. Hitherto, there are no success in using ruthenium catalysts for the reaction because of their poor catalytic performance, in spite of the fact that ruthenium is a frequently-used metallic component in hydrogenation catalysts.
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