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Bijay Shrestha on Muck Rack

Bijay Shrestha

As seen in: Archives of Pathology
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Articles

Synergistic Bimetallic Ni/Ag and Ni/Cu Catalysis for Regioselective γ,δ-Diarylation of Alkenyl Ketimines: Addressing β-H Elimination by in Situ Generation of Cationic Ni(II) Catalysts

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By Prakash Basnet, Shekhar KC, Roshan K. Dhungana, Bijay Shrestha
| American Chemical Society
We disclose unprecedented synergistic bimetallic Ni/Ag and Ni/Cu catalysts for regioselective γ,δ-diarylation of unactivated alkenes in simple ketimines with aryl halides and arylzinc reagents. The bimetallic synergy, which generates cationic Ni(II) species during reaction, promotes migratory insertion and transmetalation steps and suppresses β-H elimination and cross-coupling, the major side reactions that cause serious problems during alkene difunctionalization.
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By Shekhar KC, Roshan K. Dhungana, Bijay Shrestha, Surendra Thapa, Prakash Basnet, Ramesh Giri, Namrata Khanal, Robert W. Lebrun
| American Chemical Society
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By Prakash Basnet, Roshan K. Dhungana, Surendra Thapa, Bijay Shrestha, Shekhar KC, Jeremiah M. Sears, Ramesh Giri
| American Chemical Society
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