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Articles

Bromo-Substituted Phenylbenzothiazole Cyclometalating Ligands for the Development of Reverse Saturable Absorption Materials

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By Erica S. Knorr, Jordan Kelly, Daniel Harrison, Catherine Fabiano
| ACS Publications
1. Introduction Click to copy section linkSection link copied! Over the past decades, transition metal chromophores have attracted the attention of fields such as photoredox catalysis, (1,2) photodynamic therapy, (3) and biological sensing.
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Plasmon-Induced Hot-Carrier Excited-State Dynamics in Plasmonic Semiconductor Nanocrystals

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By Catherine Fabiano, Edward T. Nguyen, Jason E. Kuszynski, Keyou Mao
| dx.doi.org
The variance of carrier relaxation pathways for WO3–x plasmonic semiconductor nanocrystals (PSNCs) is monitored by transient absorption spectroscopy following excitation of the localized surface plasmon resonance (LSPR) versus the optical band gap (Eg,opt). Excitation of the LSPR leads to efficient hot carrier population above the Fermi level in WO3–x via Landau damping, in analogy to noble metal LSPR relaxation mechanisms.
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