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Dejuan Fa

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Articles

Modulating the Oxygen Evolution Reaction Activity of Bimetallic 2D Polymers by Substituent Effects

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By Dejuan Fa, Haonan Wu, Guangyuan Feng, Shengbin Lei
| Wiley Online Library Verified
Conflict of Interest The authors declare no conflict of interest. Supporting Information Filename Description smll202500317-sup-0001-SuppMat.pdf9.5 MB Supporting Information References 1a) , , , , , , , , , , , , , , , , , , , Science. 2024, 384, 1373; b) , , , Adv. Funct. Mater. 2013, 23, 5363; c) , , , , , , , , , , , , , , , , , , Nat. Chem. 2020, 12, 1060. 2a) , , , , , , , , , , , , , , , , , , , , Nat. Commun. 2020, 11, 2522; b) , , , , , , , , , , , , Adv. Mater. 2019, 31, 1805127; c) , , , , J.
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Regulating the Synergistic Effect in Bimetallic Two‐Dimensional Polymer Oxygen Evolution Reaction Catalysts by Adjusting the Coupling Strength Between Metal Centers

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By Dejuan Fa, Jiangyan Yuan, Guangyuan Feng, Shengbin Lei
| Wiley Online Library Verified
Graphical Abstract A series of bimetallic Co−Ni two-dimensional polymer model oxygen evolution reaction (OER) catalyst with well-defined architecture, monolayer characteristic, different metal center spacing or different conjugation degree of bridge skeleton were designed and synthesized to explore the influence of the coupling strength between metal centers for OER.
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Spatial Well‐defined Bimetallic Two‐Dimensional Polymers with Single‐Layer Thickness for Electrocatalytic Oxygen Evolution Reaction

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By Dejuan Fa, Yanhong Tao, Xin Pan, Dingjia Wang
| Wiley Online Library Verified
Abstract The well-defined architecture, identical density of active sites, and monolayer characteristic of bimetallic Ni, Co two-dimensional polymer model oxygen evolution reaction catalysts can decouple the intrinsic activity of active sites from other factors. The experimental and density functional theory simulation shown that the relative position and local coordination environment has a significant effect on the cooperation between the metal centers.
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