Eftyxis Galanos on Muck Rack

Eftyxis Galanos

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Articles

Tapered Multiblock Copolymers Based on Isoprene and 4-Methylstyrene: Influence of the Tapered Interface on the Self-Assembly and Thermomechanical Properties

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By Eftyxis Galanos, Eduard Grune, Christian Wahlen, Michael Appold
| American Chemical Society
Eftyxis Galanos†, Eduard Grune‡§, Christian Wahlen‡, Axel H. E.
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Isoprene/Styrene Tapered Multiblock Copolymers with up to Ten Blocks: Synthesis, Phase Behavior, Order, and Mechanical Properties

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By Tobias Johann, Michael Appold, Marvin Steube, Eftyxis Galanos
| American Chemical Society
The living anionic copolymerization of isoprene and styrene in cyclohexane affords tapered block copolymers due to the highly disparate reactivity ratios of rI = 12.8 and rS = 0.051. Repeated addition of a mixture of these monomers was exploited to generate tapered multiblock copolymer architectures of the (AB)n type with up to 10 blocks (1 ≤ n ≤ 5), thereby subdividing the polymer chains in alternating flexible polyisoprene (PI) and rigid polystyrene (PS) segments.
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