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Eric Matthew Ferreira on Muck Rack

Eric Matthew Ferreira

As seen in: Chemistry World
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Chromium Photocatalysis: Accessing Structural Complements to Diels-Alder Adducts with Electron-Deficient Dienophiles

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By Susan M. Stevenson, Robert F. Higgins, Matthew P Shores, Eric Matthew Ferreira
| Chemistry World Verified
A chromium-catalyzed, visible light-activated net [4+2] cycloaddition between dienes and electron-deficient alkenes is described. Gathered evidence, via control experiments, isolated intermediates, and measured redox potentials, points to several converging reaction pathways that afford the cyclohexene adducts, including a photochemical [2+2] cycloaddition/vinylcyclobutane rearrangement cascade and a substrate excitation/oxidation sequence to a radical cation intermediate.
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