Jayjit Kumar Dey

Conflicts of Interest The authors declare no conflicts of interest. Data Availability Statement The data that support the findings of this study are available from the corresponding author upon reasonable request. Supporting Information Filename Description adma72186-sup-0001-SuppMat.pdf3.4 MB Supporting File: adma72186-sup-0001-SuppMat.pdf. References 1, , , and , “Photoinduced Insulator-to-Metal Transition in a Perovskite Manganite,” Physical Review Letters 78 (1997): 4257.

Abstract The direct experimental probing and detailed imaging of octahedral tilt, along with the control of magnetic ground state and spin-orbit occupancies in an artificially engineered heterointerface through the strain manipulation via interface engineering, is the long-standing challenging issue addressed here.

Multi-step transitions between a variety of topological spin textures have been unveiled in a centrosymmetric magnet, which may enable efficient multistate memory and logic devices.