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Mitigating Voltage Decay via Chemo-Mechanical Decoupling Enabled by a Rigid-Soft Gradient Interphase in Li-Rich Layered Oxides
1 Introduction The pursuit of higher energy densities in lithium-ion batteries has intensified the search for cathode materials that transcend conventional intercalation chemistry [1]. Li‑rich layered oxides (LLOs) stand at the forefront of this endeavor, offering exceptional specific capacities exceeding 250 mAh g−1 [2, 3].
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