Kahono Shibata on Muck Rack

Kahono Shibata

As seen in: Royal Society of Chemistry
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Articles

Visible-light-induced radical switching using benzothiazolyl sulfides for geminal carbon-carbon bond formation

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By Naoya Hasegawa, Tetsuya Sengoku, Kahono Shibata, Haruto Hijikata
| Royal Society of Chemistry Verified
Visible-light-induced radical switching using benzothiazolyl sulfides for geminal carbon–carbon bond formation We propose a 2-benzothiazolylthio group as a novel auxiliary for radical switching. Using an acridinium-based photocatalyst, carbon radicals are generated from α-C–H bonds in sulfides, which are subsequently coupled with electron-deficient alkenes. This approach enables efficient access to γ,γ-disubstituted α-amino acid derivatives via two sequential photoredox reactions.
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