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Pulsed Electrolysis Promotes CO2 Electroreduction to Multicarbon Products by Suppressing Electrolyte Flooding
Conflict of Interests The authors declare no conflict of interest. Data Availability Statement The data that support the findings of this study are available from the corresponding author upon reasonable request. Supporting Information Filename Description anie70815-sup-0001-SuppMat.docx6.8 MB Supporting Information anie70815-sup-0002-Videos.zip240.3 MB Supporting Information References 1, , , , , , , Adv. Mater. 2019, 31, 1807166, https://doi.org/10.1002/adma.201807166.
Pulsed Electrolysis Promotes CO2 Electroreduction to Multicarbon Products by Suppressing Electrolyte Flooding
Electrochemical CO2 reduction (CO2RR) converts CO2 into value-added fuels and chemicals using renewable electricity. Pulsed CO2RR(p-CO2RR) has been proposed to enhance the selectivity of multicarbon products (C2+), yet mechanistic clarity at industrially relevant rates remains limited by the complex gas–liquid–solid microenvironment of gas-diffusion electrodes (GDEs). Here, we investigate p-CO2RR in GDE flow-cells operating at industrially-relevant current densities.
Recent advances in non-perfluorinated sulfonic acid proton exchange membranes in the energy field
Recent advances in non-perfluorinated sulfonic acid proton exchange membranes in the energy field The proton exchange membrane (PEM) has become one of the most popular materials for membrane-based energy conversion and storage devices due to its robust proton transport performance and high selectivity. It holds significant promise in applications such as fuel cells and electrolytic hydrogen production.
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