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Articles by Niko T Flosbach
Subzero-Temperature NMR Observation of Protein Dynamics and Ligand Binding Enabled by Encapsulation Within Coordination Cages
1 Introduction Nuclear magnetic resonance (NMR) spectroscopy has proven to be a powerful tool for investigating protein dynamics, yet motions occurring faster than the NMR timescale remain challenging to characterize [1-3]. In addition to relaxation-dispersion analyses [4, 5] and advanced pulse-sequence methodologies [6-8], lowering the temperature represents an attractive means of analyzing rapid dynamics by slowing them down enough to be observable [9-24].
High Pressure Synthesis of Pr2O5 - A Unique Lanthanoid(IV) Oxide Peroxide
The unique physical and chemical properties of the lanthanoids make them essential components in modern technologies, including electronics, optical devices, and magnetic materials.1 The chemistry of the lanthanoids is dominated by the +III oxidation state that is the most stable for all elements of the series. However, variations in the electronic configuration of lanthanoids in different oxidation states significantly influence the physical properties of their ions.
Front Cover: The Divalent Lanthanoid Triflates Ln(CF3SO3)2(CH3CN) (Ln=Sm, Eu): Structure, Luminescence, and Magnetism (Chem. Eur. J. 24/2024)
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The Divalent Lanthanoid Triflates Ln(CF3SO3)2(CH3CN) (Ln=Sm, Eu): Structure, Luminescence, and Magnetism
Introduction The chemistry of the lanthanoids is strongly stamped by the trivalent oxidation state and by the fact that the f-electrons of these elements are strongly shielded and are essentially not involved in chemical bonding.1-4 On the other hand, the well-shielded electrons lead to unique physical properties of the Ln3+-ions, and especially their luminescence and their magnetism have attracted significant attention that has led to various applications.5-9 The luminescence of most...
Competition between N and O: use of diazine N-oxides as a test case for the Marcus theory rationale for ambident reactivity
Competition between N and O: use of diazine N-oxides as a test case for the Marcus theory rationale for ambident reactivity† Kevin J. Sheehy, a Lorraine M. Bateman, abd Niko T. Flosbach,c Martin Breugst *c and Peter A.
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