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Articles by Philipp Erdmann
Critical Evaluation of Childs Method for the NMR Spectroscopic Scaling of Effective Lewis Acidity: Limitations and Resolution of Earlier Discrepancies
Supporting Information As a service to our authors and readers, this journal provides supporting information supplied by the authors. Such materials are peer reviewed and may be re-organized for online delivery, but are not copy-edited or typeset. Technical support issues arising from supporting information (other than missing files) should be addressed to the authors.
A Benchmark Study of DFT‐Computed p‐Block Element Lewis Pair Formation Enthalpies against Experimental Calorimetric Data
Supporting Information As a service to our authors and readers, this journal provides supporting information supplied by the authors. Such materials are peer reviewed and may be re-organized for online delivery, but are not copy-edited or typeset. Technical support issues arising from supporting information (other than missing files) should be addressed to the authors.
How to Deal with Charge in the Ranking of Lewis Acidity: Critical Evaluation of an Extensive Set of Cationic Lewis Acids
Introduction Lewis acids are ubiquitous reagents in chemistry, materials, and life science.1 Combining suitable acceptor atoms with appropriate ligands enables the fine-tuning of Lewis acidity to the “amount” for the desired mode of action or optimized catalytic turnover.
Predicting Lewis Acidity: Machine Learning the Fluoride Ion Affinity of p‐Block‐Atom‐Based Molecules
Introduction Lewis acids are omnipresent in all branches of chemistry, including fundamental research and synthesis, industrial-scale production, and bio-related processes.1 The fluoride ion affinity (FIA) has developed into one of the most common measures to quantitatively assess Lewis acidity in its thermodynamic sense (global Lewis acidity).2 The FIA is defined as the negative reaction enthalpy of the binding between a fluoride anion and a given Lewis acid (Figure 1A).
Trialkoxysilane Exchange: Scope, Mechanism, Cryptates and pH‐Response
Graphical Abstract The exchange reaction of trialkoxysilanes with alcohols typically requires very harsh conditions and has therefore not been used for the self-assembly of host-guest systems. In this work, unexpected solvent and salt effects are described, rationalized and exploited for the synthesis of degradable supramolecular hosts.
What Distinguishes the Strength and the Effect of a Lewis Acid: Analysis of the Gutmann-Beckett Method
Abstract What is the Gutmann–Beckett number? An experimental and theoretical evaluation of factors that determine the 31P NMR shifts of binding of 130 Lewis acids to triethylphosphine oxide allows linking the strength of a Lewis acid (global Lewis acidity) with the effect of a Lewis acid (effective Lewis acidity). Abstract IUPAC defines Lewis acidity as the thermodynamic tendency for Lewis pair formation.
A Selective Autophagy Pathway for Phase-Separated Endocytic Protein Deposits
Highlights • Ede1 is an intrinsic autophagy receptor for aberrant CME protein assemblies • Aberrant CME assemblies form by liquid-liquid phase separation • Liquid-liquid phase separation of Ede1 is important for autophagic degradation • Ultrastructural view of an LLPS compartment at the PM and within autophagic bodies Summary Autophagy eliminates cytoplasmic content selected by autophagy receptors, which link cargo to the membrane-bound autophagosomal ubiquitin-like protein Atg8/LC3.
Architecture of the centriole cartwheel‐containing region revealed by cryo‐electron tomography
Abstract Centrioles are evolutionarily conserved barrels of microtubule triplets that form the core of the centrosome and the base of the cilium. While the crucial role of the proximal region in centriole biogenesis has been well documented, its native architecture and evolutionary conservation remain relatively unexplored.
Tripartite phase separation of two signal effectors with vesicles priming B cell responsiveness
Abstract Antibody-mediated immune responses rely on antigen recognition by the B cell antigen receptor (BCR) and the proper engagement of its intracellular signal effector proteins. Src homology (SH) 2 domain-containing leukocyte protein of 65 kDa (SLP65) is the key scaffold protein mediating BCR signaling. In resting B cells, SLP65 colocalizes with Cbl-interacting protein of 85 kDa (CIN85) in cytoplasmic granules whose formation is not fully understood.
Bacterial encapsulins as orthogonal compartments for mammalian cell engineering
Mammalian codon-optimized MxEncA (UniProt:MXAN_3556) MxEncB, MxEncC, and MxEncD (UniProt: MXAN_3557, MXAN_4464, MXAN_2410) were custom synthesized by Integrated DNA Technologies and cloned into pcDNA 3.1 ( + ) Zeocin (Invitrogen) using restriction cloning or Gibson assembly. The MxEncA surface tags (FLAG or StrepTagII) were C-terminally appended using Q5® Site-Directed Mutagenesis (New England Biolabs). N-terminal Myc epitopes were added accordingly to the cargo proteins.
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