Ping Koy Lam

Abstract Non-phase-matched spontaneous parametric down-conversion (SPDC) in atomically thin materials provides new degrees of freedom and enhanced quantum information capacity compared to conventional phase-matched sources. These systems emerged as promising platforms for quantum computing, communication, and imaging, with the potential to support higher-order nonlinear processes. However, direct observation of photon-pair emission from a monolayer has remained experimentally challenging.

Abstract Quantum key distribution (QKD) provides secure communication using quantum mechanics, with continuous-variable QKD (CV-QKD) being an attractive solution due to its compatibility with existing telecommunication technology. Its main drawback is susceptibility to signal loss in fibres and free-space links, including satellites, which limits performance.

Abstract Quasi-phase matching (QPM) is a technique extensively utilized in nonlinear optics for enhancing the efficiency and stability of frequency conversion processes. However, the conventional QPM relies on periodically poled ferroelectric crystals, which are limited in availability. The 3R phase of molybdenum disulfide (3R-MoS2), a transition metal dichalcogenide (TMDc) with the broken inversion symmetry, stands out as a promising candidate for QPM, enabling efficient nonlinear process.