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X-ray Raman scattering: a building block for nonlinear spectroscopy

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By Nina Rohringer, Rohringer Nina
| royalsocietypublishing.org
1. Introduction X-ray free-electron lasers (XFELs) hold the promise to shed new light on coherent processes with resolutions down to the electronic length scale and electronic time scale. One of the great potential applications and new methodologies is the extension of nonlinear optical spectroscopy to the X-ray spectral domain. Already in the forefront of the advent of XFELs, S. Mukamel and colleagues pioneered developing concepts of nonlinear X-ray pump-probe spectroscopy [1,2].
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