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Tailoring the framework composition of carbon nitride to improve the catalytic efficiency of the stabilised palladium atoms

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By Sharon Mitchell, Evgeniya Vorobyeva, Zupeng Chen, Rowan Kendall Leary
| Royal Society of Chemistry Verified
Graphitic carbon nitride (g-C3N4) exhibits unique properties for the preparation of single-atom heterogeneous catalysts (SAHCs) due to the presence of sixfold nitrogen-based coordination sites in the lattice. Despite the potential to profoundly affect the metal stabilisation and resulting catalytic properties, no work has previously investigated the effect of modifying the carrier composition. Here, we study the impact of doping carbon in g-C3N4 on the interaction with palladium.
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