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Iridium(III) Homo- and Heterogeneous Catalysed Hydrogen Borrowing C-N Bond Formation

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By Roy Thomas McBurney, Matthew B. Peterson, John Gooding Verified, Samantha Carys Binding
| Royal Society of Chemistry Verified
Pentamethylcyclodienyl iridium(III) complexes of bidentate carbene-triazole ligands were found to be excellent homogeneous catalysts for the hydrogen borrowing mediated coupling of alcohols with amines. The reactions are highly efficient, able to reach completion in under 6 h at 100 °C at low catalyst loadings of 0.5 mol%, and are environmentally benign, the only by-product is water.
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