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Shivaiah Vaddypally

As seen in: Royal Society of Chemistry
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Articles

Transition-metal-mediated reduction and reversible double-cyclization of cyanuric triazide to an asymmetric bitetrazolate involving cleavage of the six-membered aromatic ring

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By Alex Byrne, Shivaiah Vaddypally, Vitaly G. Kiselev, C. Franklin Goldsmith
| Royal Society of Chemistry Verified
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Activation of C-H, N-H, and O-H Bonds via Proton-Coupled Electron Transfer to a Mn(III) Complex of Redox-Noninnocent Octaazacyclotetradecadiene, a Catenated-Nitrogen Macrocyclic Ligand - Journal of the American Chemical Society (ACS Publications)

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By Shivaiah Vaddypally, Warren Tomlinson, Owen T. O’Sullivan, Ran Ding
| American Chemical Society
Shivaiah Vaddypally† , Warren Tomlinson‡, Owen T. O’Sullivan†, Ran Ding† , Megan M. Van Vliet† , Bradford B. Wayland†, Joseph P. Hooper*‡ , and Michael J. Zdilla*† † Department of Chemistry, Temple University, 1901 North 13th Street, Philadelphia, Pennsylvania 19122 , United States ‡ Department of Physics, Naval Postgraduate School, 833 Dyer Road, Monterey, California 93943 , United States J. Am. Chem.
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Reactive Pendant Mn═O in a Synthetic Structural Model of a Proposed S4 State in the Photosynthetic Oxygen Evolving Complex

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By Shivaiah Vaddypally, Sandeep K. Kondaveeti, Santosh Karki, Robert J. Levis
| American Chemical Society
The molecular mechanism of the Oxygen Evolving Center of photosystem II has been under debate for decades. One frequently cited proposal is the nucleophilic attack by water hydroxide on a pendant Mn?O moiety, though no chemical example of this reactivity at a manganese cubane cluster has been reported. We describe here the preparation, characterization, and a reactivity study of a synthetic manganese cubane cluster with a pendant manganese-oxo moiety.
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