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Close-space sublimation as a versatile deposition process for efficient perovskite silicon tandem solar cells
Abstract The envisaged breakthrough of perovskite photovoltaic technologies demands rapid advances in scalable and robust high-throughput fabrication methods. Here we present close-space sublimation (CSS) as a vacuum-based, industrially relevant deposition method for the conversion of sublimed PbI2 inorganic scaffolds into high-quality wide-bandgap perovskite absorbers (MAPb(I0.79Br0.21)3, 1.64 eV), employing a reusable mixed-halide organic source for stable bandgap control.
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