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Tomas J. Saiegh on Muck Rack

Tomas J. Saiegh

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Articles

Cyclic Diaryl λ3‐Bromanes as a Precursor for Regiodivergent Alkynylation Reactions

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By Maxime de Abreu, Torben Rogge, Matteo Lanzi, Tomas J. Saiegh
| Wiley Online Library Verified
Rapid construction of molecular complexity under mild and sustainable conditions is one of the key challenges of modern synthetic chemistry.
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Light‐Driven Alkyne gem‐Hydrogenation: An Intramolecular Approach to Hoveyda‐Grubbs Catalysts

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By Tomas J. Saiegh, Tobias Biberger, Raphael J. Zachmann, Alois Fürstner
| Wiley Online Library Verified
Abstract The light-driven gem-hydrogenation of internal alkynes in the presence of [(NHC)(η6-cymene)RuCl2] generates discrete ruthenium carbene complexes. When applied to appropriately designed enyne substrates, the reactive intermediates thus formed will engage the tethered olefin in metathetic ring closure while splitting off a Hoveyda-Grubbs-type complex as secondary carbene.
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