Trimbak Baliram Mete on Muck Rack

Trimbak Baliram Mete

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Articles

Conformation-driven reversibility control in ring-opening metathesis polymerization of non-bicyclic cyclooctenes - Nature Communications

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By Kyungmin Choi, Seulchan Lee, Hajime Hirao, Trimbak Baliram Mete
| Nature Verified
Abstract Reversible ring-opening metathesis polymerization (ROMP) of cyclooctene (COE) derivatives remains a challenge due to their high ring strain energies (RSEs). While previous strategies rely on fused bicyclic systems to reduce RSEs, depolymerization of non-bicyclic COE polymers has proven difficult. Here, we demonstrate efficient reversible ROMP of non-bicyclic COE derivatives by introducing conformational constraints via geminal tert-butyl and hydroxy substituents.
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